News
New Publication “Nanoantenna design for enhanced carrier–envelope-phase sensitivity”
Optical-field emission from nanostructured solids such as subwavelength nanoantennas can be leveraged to create sub-femtosecond, petahertz-scale electronics for optical-field detection. One application of particular interest is the detection of an incident optical pulse’s carrier–envelope phase (CEP). Such CEP detection requires few-cycle, broadband optical excitation where the resonant properties of the nanoantenna can strongly alter the response of the near field in time. Little quantitative investigation has been performed to understand how the geometry and resonant properties of the antennas should be tuned to enhance the CEP sensitivity and signal-to-noise ratio. Here we examine how the geometry and resonance frequency of planar plasmonic nanoantennas can be engineered to enhance the emitted CEP-sensitive photocurrent when driven by a few-cycle optical pulse. We find that with the simple addition of curved sidewalls leading to the apex, and proper tuning of the resonance wavelength, the net CEP-sensitive current per nanoantenna can be improved by 5−10×, and the signal-to-noise-ratio by 50−100× relative to simple triangular antennas operated on resonance. Our findings will inform the next generation of nanoantenna designs for emerging applications in ultrafast photoelectron metrology and petahertz electronics.
A complete description of the work may be found here.
Marco Colangelo awarded IEEE CSC fellowship
Congratulations to Marco Colangelo on receiving the IEEE CSC Graduate Study Fellowship in Applied Superconductivity.
New Publication “Electrostatic electron mirror in SEM for simultaneous imaging of top and bottom surfaces of a sample”
The use of electron mirrors in aberration correction and surface-sensitive microscopy techniques such as low-energy electron microscopy has been established. However, in this work, by implementing an easy to construct, fully electrostatic electron mirror system under a sample in a conventional scanning electron microscope (SEM), we present a new imaging scheme which allows us to form scanned images of the top and bottom surfaces of the sample simultaneously. We believe that this imaging scheme could be of great value to the field of in-situ SEM which has been limited to observation of dynamic changes such as crack propagation and other surface phenomena on one side of samples at a time. We analyze the image properties when using a flat versus a concave electron mirror system and discuss two different regimes of operation. In addition to in-situ SEM, we foresee that our imaging scheme could open up avenues towards spherical aberration correction by the use of electron mirrors in SEMs without the need for complex beam separators.
A complete description of the work may be found here.
New Publication “Nanoscale refractory doped titanium nitride field emitters”
Refractory materials exhibit high damage tolerance, which is attractive for the creation of nanoscale field-emission electronics and optoelectronics applications that require operation at high peak current densities and optical intensities. Recent results have demonstrated that the optical properties of titanium nitride, a refractory and CMOS-compatible plasmonic material, can be tuned by adding silicon and oxygen dopants. However, to fully leverage the potential of titanium (silicon oxy)nitride, a reliable and scalable fabrication process with few-nm precision is needed. In this work, we developed a fabrication process for producing engineered nanostructures with gaps between 10 and 15 nm, aspect ratios larger than 5 with almost 90° steep sidewalls. Using this process, we fabricated large-scale arrays of electrically-connected bow-tie nanoantennas with few-nm free-space gaps. We measured a typical variation of 4 nm in the average gap size. Using applied DC voltages and optical illumination, we tested the electronic and optoelectronic response of the devices, demonstrating sub-10-V tunneling operation across the free-space gaps, and quantum efficiency of up to 1centerdot10-3 at 1.2 μm, which is comparable to a bulk silicon photodiode at the same wavelength and three orders of magnitude higher than with nearly identical gold devices. Tests demonstrated that the titanium silicon oxynitride nanostructures did not significantly degrade, exhibiting less than 5 nm of shrinking of the average gap dimensions over few-μm2 areas after 10 hours of operation. Our results will be useful for developing the next generation of robust and CMOS-compatible nanoscale devices for high-speed and low-power field-emission electronics and optoelectronics applications.
A complete description of the work may be found here.
New Publication “On-chip sampling of optical fields with attosecond resolution”
We demonstrate an on-chip, optoelectronic device capable of sampling arbitrary, low-energy, near-infrared waveforms under ambient conditions with sub-optical-cycle resolution. Our detector uses field-driven photoemission from resonant nanoantennas to create attosecond electron bursts that probe the electric field of weak optical waveforms. Using these devices, we sampled the electric fields of ~5 fJ (6.4 MV m−1), few-cycle, near-infrared waveforms using ~50 pJ (0.64 GV m−1) near-infrared driving pulses. Beyond sampling these weak optical waveforms, our measurements directly reveal the localized plasmonic dynamics of the emitting nanoantennas in situ. Applications include broadband time-domain spectroscopy of molecular fingerprints from the visible region through the infrared, time-domain analysis of nonlinear phenomena and detailed investigations of strong-field light–matter interactions.
A complete description of the work may be found here.
